DIGPEDI has been releasing 4k versions of several LOONA MVs on their Vimeo account since July 15th. Some of these MVs have been on their account for a while, however, the 4k quality versions were not available until recently. Others are just being uploaded to their Vimeo account for the first time after previously only being available via the loonatheworld YouTube channel. For those unfamiliar, DIGIPEDI is LOONA's go-to video director (they've handled most of LOONA's music video releases since Hyunjin's solo in late 2016).
So far they have released 4k versions of:
Around You (Original Film Ver.)
Kiss Later
Heart Attack
Love&Live
Girl Front
Sweet Crazy Love
Hi High
Butterfly
It seems like they've been releasing at least one 4k version per day, but it seems to be pretty random (not in release order). Hopefully they'll eventually release 4k versions of all of the MVs they've created with LOONA!
So far they have released 4k versions of:
Around You (Original Film Ver.)
Kiss Later
Heart Attack
Love&Live
Girl Front
Sweet Crazy Love
Hi High
Butterfly
It seems like they've been releasing at least one 4k version per day, but it seems to be pretty random (not in release order). Hopefully they'll eventually release 4k versions of all of the MVs they've created with LOONA!
I'm sad I want to watch them but my computer is too old to run 4K smoothly 
mine can barely handle themI'm sad I want to watch them but my computer is too old to run 4K smoothly
someday i will get a fancy 4k tv or something
Girl Front in 4K is a whole new experience omfg
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woah 
favOriTe and Everyday I Love You also have 4k versions now too:
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oh wow- nice